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Cu(In 4

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Photosynthesis and related metabolic mechanism of promoted rice (Oryza sativai> L.) growth by TiO2sub> nanoparticles

Yingdan Zhang, Na Liu, Wei Wang, Jianteng Sun, Lizhong Zhu

《环境科学与工程前沿（英文）》 2020年第14卷第6期 doi: 10.1007/s11783-020-1282-5

摘要： Abstract • The rice growth was promoted by nano-TiO2 of 0.1–100 mg/L. • Nano-TiO2 enhanced the energy storage in photosynthesis. • Nano-TiO2 reduced energy consumption in carbohydrate metabolism and TCA cycle. Titanium dioxide nanoparticle (nano-TiO2), as an excellent UV absorbent and photo-catalyst, has been widely applied in modern industry, thus inevitably discharged into environment. We proposed that nano-TiO2 in soil can promote crop yield through photosynthetic and metabolic disturbance, therefore, we investigated the effects of nano-TiO2 exposure on related physiologic-biochemical properties of rice (Oryza sativa L.). Results showed that rice biomass was increased >30% at every applied dosage (0.1–100 mg/L) of nano-TiO2. The actual photosynthetic rate (Y(II)) significantly increased by 10.0% and 17.2% in the treatments of 10 and 100 mg/L respectively, indicating an increased energy production from photosynthesis. Besides, non-photochemical quenching (Y(NPQ)) significantly decreased by 19.8%–26.0% of the control in all treatments respectively, representing a decline in heat dissipation. Detailed metabolism fingerprinting further revealed that a fortified transformation of monosaccharides (D-fructose, D-galactose, and D-talose) to disaccharides (D-cellobiose, and D-lactose) was accompanied with a weakened citric acid cycle, confirming the decrease of energy consumption in metabolism. All these results elucidated that nano-TiO2 promoted rice growth through the upregulation of energy storage in photosynthesis and the downregulation of energy consumption in metabolism. This study provides a mechanistic understanding of the stress-response hormesis of rice after exposure to nano-TiO2, and provides worthy information on the potential application and risk of nanomaterials in agricultural production.
关键词： Nano-TiO₂ Rice Photosynthesis Metabolomics Energy storage

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用高光谱发光法研究Cu(Inxi>sub>,Ga1–xi>sub>)Se2sub> (CIGS)模块中由P1引起的功率损耗的成因 Article

César Omar Ramírez Quiroz, Laura-Isabelle Dion-Bertrand, Christoph J. Brabec, Joachim Müller, Kay Orgassa

《工程（英文）》 2020年第6卷第12期 页码 1395-1402 doi: 10.1016/j.eng.2019.12.019

摘要：
在本文中，我们利用了高光谱高分辨率光致发光映射技术，这是一个强大的工具，可用于选择和优化在Cu(Inxsub>,Ga1-xsub>)Se2sub>（CIGS）模块上对子电池进行图案化互连的激光烧蚀工艺。具体而言，通过分析在CIGS沉积之前烧蚀的标准P1图案线，我们发现了沿着下部的钼槽边缘的异常发射猝灭效应。通过扫描电子显微镜（SEM）比较了P1边缘的横截面的形貌，我们进一步合理化产生这种效应的起因，但无法用厚度变化解释光发射的减少。我们还研究了激光诱导对CIGS沉积后的P1图案线带来的损伤。我们的发现能更好地理解P1引起的功率损耗，并为改进与行业相关的模块互连方案提供了新的见解。

关键词： Cu(Inx Ga1–x)Se2 电池到模块的效率差距 由P1引起的功率损耗 高光谱光致发光 激光烧蚀短程热效应

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Superior performance in visible-light-driven hydrogen evolution reaction of three-dimensionally ordered macroporous SrTiO decorated with ZnCdS

《化学科学与工程前沿（英文）》 2021年第15卷第6期 页码 1561-1571 doi: 10.1007/s11705-021-2089-z

摘要： It is of broad interest to develop emerging photocatalysts with excellent light-harvesting capacity and high charge carrier separation efficiency for visible light photocatalytic hydrogen evolution reaction. However, achieving satisfying hydrogen evolution efficiency under noble metal-free conditions remains challenging. In this study, we demonstrate the fabrication of three-dimensionally ordered macroporous SrTiO₃ decorated with Zn_xCd₁₋_xS nanoparticles for hydrogen production under visible light irradiation (λ>420 nm). Synergetic enhancement of photocatalytic activity is achieved by the slow photon effect and improved separation efficiency of photogenerated charge carriers. The obtained composites could afford very high hydrogen production efficiencies up to 19.67 mmol·g⁻¹·h⁻¹, with an apparent quantum efficiency of 35.9% at 420 nm, which is 4.2 and 23.9 times higher than those of pure Zn_0.5Cd_0.5S (4.67 mmol·g⁻¹·h⁻¹) and CdS (0.82 mmol·g⁻¹·h⁻¹), respectively. In particular, under Pt-free conditions, an attractive hydrogen production rate (3.23 mmol·g⁻¹·h⁻¹) was achieved, providing a low-cost and high-efficiency strategy to produce hydrogen from water splitting. Moreover, the composites showed excellent stability, and no obvious loss in activity was observed after five cycling tests.

关键词： three-dimensionally ordered macroporous SrTiO₃ Zn_xCd_1–_xS visible light hydrogen production promotion mechanism

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磁控溅射法生长的带隙可调谐(GaxIn1−x)2O3 Research Articles

张法碧1,孙巾寓1,李海鸥1,周娟1,王荣1,孙堂友1,傅涛1,肖功利1,李琦1,刘兴鹏1,张秀云1,郭道友2,王相虎3,秦祖军1

《信息与电子工程前沿（英文）》 2021年第22卷第10期 页码 1370-1378 doi: 10.1631/FITEE.2000330

摘要：采用磁控溅射技术和热退火技术在(0001)蓝宝石衬底上制备了多组分氧化物(GaxIn1−x)2O3薄膜，实现可调带隙。详细研究了三元化合物(GaxIn1−x)2O3在整个组成范围内的光学性质和能带结构演化。X射线衍射谱表明，Ga含量在0.11至0.55之间的(GaxIn1−x)2O3薄膜既有立方结构，也有单斜结构，而Ga含量高于0.74的(GaxIn1−x)2O3薄膜只有单斜结构。实验结果为透明导电化合物半导体(GaxIn1−x)2O3薄膜在光电和光伏行业的应用，特别是在显示器、发光二极管和太阳能电池的应用奠定了基础。

关键词： (GaxIn1−x)2O3薄膜；带隙可调谐；磁控溅射

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NiFeRuOxi>sub> nanosheets on Ni foam as an electrocatalyst for efficient

《化学科学与工程前沿（英文）》 2023年第17卷第11期 页码 1698-1706 doi: 10.1007/s11705-023-2334-8

摘要： The electrocatalyst NiFeRuO_x/NF, comprised of NiFeRuO_x nanosheets grown on Ni foam, was synthesized using a hydrothermal process followed by thermal annealing. NiFeRuO_x/NF displays high electrocatalytic activity and stability for overall alkaline seawater splitting: 98 mV@ 10 mA∙cm⁻² in hydrogen evolution reaction, 318 mV@ 50 mA∙cm⁻² in oxygen evolution reaction, and a cell voltage of 1.53 V@ 10 mA∙cm⁻², as well as 20 h of durability. A solar-driven system containing such a bifunctional NiFeRuO_x/NF has an almost 100% Faradaic efficiency. The NiFeRuO_x coating around Ni foam is an anti-corrosion layer and also a critical factor for enhancement of bifunctional performances.

关键词： NiFeRuO_x nanosheets Ni foam electrocatalysis overall seawater splitting solar-driven system

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H2sub> 对Pt-Ba-Ce /γ-Al2sub>O3sub> 催化剂NOxi>sub> 存储和还原机理的影响研究 Article

王攀, 裔静, 孙川, 罗鹏, 雷利利

《工程（英文）》 2019年第5卷第3期 页码 568-575 doi: 10.1016/j.eng.2019.02.005

摘要：
本研究采用浸渍法制备了Pt-Ba-Ce/γ-Al2sub>O3sub>催化剂，利用实验评价了H2sub> 对NSR（NOxsub> storage and reduction）催化剂存储和还原机理的影响，并采用综合表征技术研究了Pt-Ba-Ce /γ-Al2sub>O3sub结果表明，透射电子显微镜（TEM）显示X 射线衍射（XRD）光谱中观察到的PtOxsub>、CeO2sub> 和BaCO3sub> 峰很好地分散在在NOxsub> 完全存储- 还原实验中，NO2sub> 产量的增加使NOxsub> 的存储能力在250~350 ℃ 的温度范围内大大提高，在350 ℃ 达到最大值315.3 μmol·g^–1。

关键词： Pt–Ba–Ce/γ-Al2sub>O3sub> 催化剂，物理化学性质，NOxi>sub>存储和还原，NOxi>sub> 排放，H2sub> 还原剂

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NOxi>sub> and H2sub>S formation in the reductive zone of air-staged combustion of

Jinzhi CAI, Dan LI, Denggao CHEN, Zhenshan LI

《能源前沿（英文）》 2021年第15卷第1期 页码 4-13 doi: 10.1007/s11708-020-0804-y

摘要： Low NO combustion of blended coals is widely used in coal-fired boilers in China to control NO emission; thus, it is necessary to understand the formation mechanism of NO and H S during the combustion of blended coals. This paper focused on the investigation of reductive gases in the formation of NO and H S in the reductive zone of blended coals during combustion. Experiments with Zhundong (ZD) and Commercial (GE) coal and their blends with different mixing ratios were conducted in a drop tube furnace at 1200°C–1400°C with an excessive air ratio of 0.6–1.2. The coal conversion and formation characteristics of CO, H S, and NO in the fuel-rich zone were carefully studied under different experimental conditions for different blend ratios. Blending ZD into GE was found to increase not only the coal conversion but also the concentrations of CO and H S as NO reduction accelerated. Both the CO and H S concentrations inblended coal combustion increase with an increase in the combustion temperature and a decrease in the excessive air ratio. Based on accumulated experimental data, one interesting finding was that NO and H S from blended coal combustion were almost directly dependent on the CO concentration, and the CO concentration of the blended coal combustion depended on the single char gasification conversion.Thus, CO, NO , and H S formation characteristics from blended coal combustion can be well predicted by single char gasification kinetics.

关键词： blended coal combustion NO_xformation H₂S formation air staged combustion

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通过 B i>位Ta置换对 AB i> O4sub>型EuNbO4sub>的热学和力学性质进行优化 Article

陈琳, 冯晶

《工程（英文）》 2020年第6卷第2期 页码 177-184 doi: 10.1016/j.eng.2019.12.006

摘要：
铁弹性的ABO4sub>型RETaO4sub>陶瓷和RENbO4sub>陶瓷（RE表示稀土）是具有潜在应用价值的热障涂层（TBC）材料，结果显示， RETaO4sub>陶瓷的力学性质优于RENbO4sub>陶瓷的力学性质。在本研究中，我们通过B位钽（Ta）置换对利用固相法（SSR）制备的EuNbO4sub>陶瓷的热学和力学性质进行优化。;5 K⁻¹（1200 ℃）； EuNbO4sub>陶瓷的热导率被降低至1.52 W·K^–1·m^–1（700 ℃），且材料的抗热辐射能力得到了改善。

关键词：热障涂层，稀土铌酸盐，置换，热导率，热膨胀系数，杨氏模量

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Accounting for the uncertainties in the estimation of average shear wave velocity using – correlations

《结构与土木工程前沿（英文）》 2021年第15卷第5期 页码 1199-1208 doi: 10.1007/s11709-021-0749-1

摘要： Site-specific seismic hazard analysis is crucial for designing earthquake resistance structures, particularly in seismically active regions. Shear wave velocity ( V _S) is a key parameter in such analysis, although the economy and other factors restrict its direct field measurement in many cases. Various V _S–SPT– N correlations are routinely incorporated in seismic hazard analysis to estimate the value of V _S. However, many uncertainties question the reliability of these estimated V _S values. This paper comes up with a statistical approach to take care of such uncertainties involved in V _S calculations. The measured SPT– N values from all the critical boreholes were converted into statistical parameters and passed through various correlations to estimate V _S at different depths. The effect of different soil layers in the boreholes on the Vs estimation was also taken into account. Further, the average shear wave velocity of the top 30 m soil cover ( V _S30) is estimated after accounting for various epistemic and aleatoric uncertainties. The scattering nature of the V _S values estimated using different V _S– N correlations was reduced significantly with the application of the methodology. Study results further clearly demonstrated the potential of the approach to eliminate various uncertainties involved in the estimation of V _S30 using general and soil-specific correlations.

关键词： uncertainties V _S– N correlations V _S30 SPT data statistical methodology

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CeO doping boosted low-temperature NH-SCR activity of FeTiO catalyst: A microstructure analysis and reaction mechanistic study

《环境科学与工程前沿（英文）》 2022年第16卷第5期 doi: 10.1007/s11783-022-1539-2

摘要：
• CeO₂ doping significantly improved low-temperature NH₃-SCR activity on FeTiO_x.

关键词： NH₃-SCR CeO₂ doping Low-temperature NO_x removal Improved redox property In situ XAFS analysis

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Chemical poison and regeneration of SCR catalysts for NOxi>sub>

Junhua LI,Yue PENG,Huazhen CHANG,Xiang LI,John C. CRITTENDEN,Jiming HAO

《环境科学与工程前沿（英文）》 2016年第10卷第3期 页码 413-427 doi: 10.1007/s11783-016-0832-3

摘要： Selective catalytic reduction (SCR) of NO with NH is an effective technique to remove NO from stationary sources, such as coal-fired power plant and industrial boilers. Some of elements in the fly ash deactivate the catalyst due to strong chemisorptions on the active sites. The poisons may act by simply blocking active sites or alter the adsorption behaviors of reactants and products by an electronic interaction. This review is mainly focused on the chemical poisoning on V O -based catalysts, environmental-benign catalysts and low temperature catalysts. Several common poisons including alkali/alkaline earth metals, SO and heavy metals etc. are referred and their poisoning mechanisms on catalysts are discussed. The regeneration methods of poisoned catalysts and the development of poison-resistance catalysts are also compared and analyzed. Finally, future research directions in developing poisoning resistance catalysts and facile efficient regeneration methods for SCR catalysts are proposed.

关键词： flue gas DeNO_x SCR catalyst poison and regeneration

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Recent advances in special morphologic photocatalysts for NO removal

《环境科学与工程前沿（英文）》 2022年第16卷第11期 doi: 10.1007/s11783-022-1573-0

摘要：
● Systematic information of recent progress in photocatalytic NO_x removal is provided.

关键词： NO_x removal Photocatalyst Graphene C₃N₄ Bi-based compounds.

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Magnetic Co-doped 1D/2D structured -FeO/MoS effectively activated peroxymonosulfate for efficient abatement

《环境科学与工程前沿（英文）》 2023年第18卷第3期 doi: 10.1007/s11783-024-1797-2

摘要：
● Magnetic Co- γ -Fe₂O₃/MoS₂ were prepared via facile hydrothermal methods.

关键词： Magnetic Co-γ-Fe₂O₃/MoS₂ Hydrothermal method Bisphenol A Degradation pathways Toxicity analysis

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Tailoring the simultaneous abatement of methanol and NO on Sb-Ce-Zr catalysts via copper modification

《环境科学与工程前沿（英文）》 2022年第16卷第10期 doi: 10.1007/s11684-022-1565-0

摘要：
● Cu addition enhances CH₃OH oxidation and alleviates its inhibitory effect on SCR.

关键词： Copper modification Sb-CeZr₂O_x catalyst NO_x Methanol Simultaneous removal

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Ni>-Positive ion activated rapid addition and mitochondrial targeting ratiometric fluorescent probesfor in vivoi> cell H2sub>S imaging

Yan Shi, Fangjun Huo, Yongkang Yue, Caixia Yin

《化学科学与工程前沿（英文）》 2022年第16卷第1期 页码 64-71 doi: 10.1007/s11705-021-2048-8

摘要： Heterocyclic compound quinoline and its derivatives exist in natural compounds and have a broad spectrum of biological activity. They play an important role in the design of new structural entities for medical applications. Similarly, indoles and their derivatives are found widely in nature. Amino acids, alkaloids and auxin are all derivatives of indoles, as are dyes, and their condensation with aldehydes makes it easy to construct reaction sites for nucleophilic addition agents. In this work, we combine these two groups organically to construct a rapid response site (within 30 s) for H S, and at the same time, a ratiometric fluorescence response is presented throughout the process of H S detection. As such, the lower detection limit can reach 55.7 nmol/L for H S. In addition, cell imaging shows that this probe can be used for the mitochondrial targeted detection of endogenous and exogenous H S. Finally, this probe application was verified by imaging H S in nude mice.

关键词： heterocyclic compound hydrogen sulfide ratiometric mitochondrial targeted

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标题作者时间类型操作

Photosynthesis and related metabolic mechanism of promoted rice (Oryza sativai> L.) growth by TiO2sub> nanoparticles
Yingdan Zhang, Na Liu, Wei Wang, Jianteng Sun, Lizhong Zhu

期刊论文



用高光谱发光法研究Cu(Inxi>sub>,Ga1–xi>sub>)Se2sub> (CIGS)模块中由P1引起的功率损耗的成因

César Omar Ramírez Quiroz, Laura-Isabelle Dion-Bertrand, Christoph J. Brabec, Joachim Müller, Kay Orgassa

期刊论文



Superior performance in visible-light-driven hydrogen evolution reaction of three-dimensionally ordered macroporous SrTiO decorated with ZnCdS

期刊论文



磁控溅射法生长的带隙可调谐(GaxIn1−x)2O3

张法碧1,孙巾寓1,李海鸥1,周娟1,王荣1,孙堂友1,傅涛1,肖功利1,李琦1,刘兴鹏1,张秀云1,郭道友2,王相虎3,秦祖军1

期刊论文



NiFeRuOxi>sub> nanosheets on Ni foam as an electrocatalyst for efficient

期刊论文



H2sub> 对Pt-Ba-Ce /γ-Al2sub>O3sub> 催化剂NOxi>sub> 存储和还原机理的影响研究

王攀, 裔静, 孙川, 罗鹏, 雷利利

期刊论文



NOxi>sub> and H2sub>S formation in the reductive zone of air-staged combustion of

Jinzhi CAI, Dan LI, Denggao CHEN, Zhenshan LI

期刊论文



通过 B i>位Ta置换对 AB i> O4sub>型EuNbO4sub>的热学和力学性质进行优化

陈琳, 冯晶

期刊论文



Accounting for the uncertainties in the estimation of average shear wave velocity using – correlations

期刊论文



CeO doping boosted low-temperature NH-SCR activity of FeTiO catalyst: A microstructure analysis and reaction mechanistic study

期刊论文



Chemical poison and regeneration of SCR catalysts for NOxi>sub>

Junhua LI,Yue PENG,Huazhen CHANG,Xiang LI,John C. CRITTENDEN,Jiming HAO

期刊论文



Recent advances in special morphologic photocatalysts for NO removal

期刊论文



Magnetic Co-doped 1D/2D structured -FeO/MoS effectively activated peroxymonosulfate for efficient abatement

期刊论文



Tailoring the simultaneous abatement of methanol and NO on Sb-Ce-Zr catalysts via copper modification

期刊论文



Ni>-Positive ion activated rapid addition and mitochondrial targeting ratiometric fluorescent probesfor in vivoi> cell H2sub>S imaging

Yan Shi, Fangjun Huo, Yongkang Yue, Caixia Yin

期刊论文